We investigate, using numerical simulations, the conformations of isolated active ring polymers. We find that their behavior depends crucially on their size: Short rings (N≲100) swell, whereas longer rings (N≳200) collapse, at sufficiently high activity. By investigating the nonequilibrium process leading to the steady state, we find a universal route driving both outcomes; we highlight the central role of steric interactions, at variance with linear chains, and of topology conservation. We further show that the collapsed rings are arrested by looking at different observables, all underlining the presence of an extremely long timescales at the steady state, associated with the internal dynamics of the collapsed section. Finally, we found that in some circumstances the collapsed state spins about its axis.

Activity-Induced Collapse and Arrest of Active Polymer Rings

Locatelli E.;
2021

Abstract

We investigate, using numerical simulations, the conformations of isolated active ring polymers. We find that their behavior depends crucially on their size: Short rings (N≲100) swell, whereas longer rings (N≳200) collapse, at sufficiently high activity. By investigating the nonequilibrium process leading to the steady state, we find a universal route driving both outcomes; we highlight the central role of steric interactions, at variance with linear chains, and of topology conservation. We further show that the collapsed rings are arrested by looking at different observables, all underlining the presence of an extremely long timescales at the steady state, associated with the internal dynamics of the collapsed section. Finally, we found that in some circumstances the collapsed state spins about its axis.
File in questo prodotto:
File Dimensione Formato  
Activity-Induced Collapse and Arrest of Active Polymer Rings.pdf

Accesso riservato

Tipologia: Published (publisher's version)
Licenza: Accesso privato - non pubblico
Dimensione 1.06 MB
Formato Adobe PDF
1.06 MB Adobe PDF Visualizza/Apri   Richiedi una copia
2103.01329v1.pdf

accesso aperto

Tipologia: Preprint (submitted version)
Licenza: Altro
Dimensione 7.71 MB
Formato Adobe PDF
7.71 MB Adobe PDF Visualizza/Apri
Pubblicazioni consigliate

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11577/3395209
Citazioni
  • ???jsp.display-item.citation.pmc??? 0
  • Scopus 60
  • ???jsp.display-item.citation.isi??? 61
  • OpenAlex ND
social impact